| 01. | Overture - Orchestra & chorus | |
| 02. | The Perfect Nanny - Karen Dotrice & Matthew Garber | |
| 03. | Sister Suffragette - Glynis Johns | |
| 04. | The Life I Lead - David Tomlinson | |
| 05. | A Spoonful of Sugar - Julie Andrews | |
| 06. | Pavement Artist (Chim Chim Cheree) - Dick Van Dyke | |
| 07. | Jolly Holliday - Dick Van Dyke & Julie Andrews | |
| 08. | Super-Cali-Fragil-istic-Expi-Ali-Docious - Julie Andrews, Dick Van Dyke & Pearlies | |
| 09. | Stay Awake - Julie Andrews | |
| 10. | I Love to Laugh - Ed Wynn & Julie Andrews | |
| 11. | A British Bank (The Life I Lead reprise) - David Tomlinson & Julie Andrews | |
| 12. | Feed the Birds (Tuppence a Bag) - Julie Andrews & chorus | |
| 13. | Fidelity Fiduciary Bank - Dick Van Dyke & David Tomlinson | |
| 14. | Chim Chim Cheree - Dick Van Dyke, Julie Andrews, Karen Dotrice, Matthew Garber | |
| 15. | Step in Time - Dick Van Dyke | |
| 16. | A Man Has Dreams (The Life I Lead/Spoonful of Sugar reprise) - David Tomlinson & Dick Van Dyke | |
| 17. | Let's Go Fly a Kite - David Tomlinson, Dick Van Dyke, chorus | |